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• W2023890969 abstract "Femtosecond transient absorption has been used to study the mechanism and dynamics of the quenching of an aromatic thioketone, 4H-1-benzopyrane-4-thione (BPT), in the S2 state, by saturated hydrocarbons (n-hexane, dodecane, hexadecane, cyclohexane, cyclohexane-d12). The results demonstrate the involvement of the hydrocarbon C–H bonds in the quenching process. Two quenching mechanisms are proposed: efficient H-atom abstraction followed by ultrafast back hydrogen transfer, or ‘aborted hydrogen abstraction’. In the latter case, the progress along the reaction path to a conical intersection is assumed to deactivate the S2 state through transition to the S1 state energy surface." @default.
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• W2023890969 date "2003-01-01" @default.
• W2023890969 modified "2023-09-26" @default.
• W2023890969 title "Nature of the S2-state quenching process of benzopyranthione by hydrocarbon solvents measured by pico- and femtosecond laser spectroscopy" @default.
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• W2023890969 doi "https://doi.org/10.1016/s0009-2614(02)01926-7" @default.
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