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- W2023936657 abstract "Abstract A series of T‐ and H‐shaped donor–acceptor (D–A) types of dipyrido[3,2‐ a :2′,3′‐ c ]phenazine (DPPZ)‐based molecules, extended by thienyl and triphenylamino chromophores at the 2,7‐(bottom) and/or 10,13‐positions (top), have been designed and prepared successfully. Synthetic, structural, thermal, spectral, and computational comparisons have been carried out for related compounds because of their adjustable intramolecular charge‐transfer properties. It is noted that a pair of structural isomers ( 5 and 6 ) has been obtained, respectively, where distinguishable UV/Vis and fluorescence spectra, electrochemical activity, thermal stability, and bandgaps are observed. Furthermore, compounds 6 , 8 , 10 , 11 , 13 , and 15 exhibit excellent thermal stability, and the Td 10 values for them are found to range from 524 to 646 °C, which can be regarded as one of the best groups of thermally stable compounds among organic small molecules. In addition, theoretical calculations were performed, and the structure–property relationships were examined to reveal the effects of the position and number of donor arms on the DPPZ acceptor core." @default.
- W2023936657 created "2016-06-24" @default.
- W2023936657 creator A5014357385 @default.
- W2023936657 creator A5024895996 @default.
- W2023936657 creator A5052342599 @default.
- W2023936657 creator A5054039263 @default.
- W2023936657 creator A5086786113 @default.
- W2023936657 creator A5090562941 @default.
- W2023936657 date "2013-11-11" @default.
- W2023936657 modified "2023-10-18" @default.
- W2023936657 title "Dipyrido[3,2-<i>a</i>:2′,3′-<i>c</i>]phenazine-Based Donor-Acceptor Aromatic Heterocyclic Compounds with Thienyl and Triphenylamino Chromophores at the 2,7- and/or 10,13-Positions" @default.
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