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- W2023943059 abstract "The frequency spectra of the linear and third nonlinear permittivities, ε 1 * and ε 3 * , have been measured for polyvinyl acetate (PVAc) at temperatures above T g . The Debye relaxation of ε 1 * associated with the micro-Brownian motion of noncrystalline segments is found to be accompanied by the complex frequency dependence of ε 3 * due to combined contributions from the intrinsic nonlinear dielectricity and the electrostriction. Additional measurements for the elastic compliance s * allow subtraction of the latter contribution (propt s * ε 1 *2 ) to yield the intrinsic nonlinear dielectric relaxation spectra in the form of Δε 3 /(1+iωτ 3 ) 3 in accordance with phenomenological prediction. The evaluated relaxation strengths, Δε 1 and Δε 3 , lead to estimates of equivalent Langevin dipoles consisting of eleven monomers and a saturation polarization of 20 mC/m 2 ." @default.
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- W2023943059 title "Nonlinear Dielectric Relaxation Spectra of Polyvinyl Acetate" @default.
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