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- W2023996779 abstract "► Review of the experimental approach for investigating gases, liquids, and solutions with soft X-ray techniques. ► Gas and liquid cells as well as a high-resolution, high-transmission X-ray spectrometer are discussed. ► By using some examples, we show how detailed information about the electronic structure of liquids, and gases is gained. We summarize our development of instrumentation for the study of liquids, aqueous solutions, and liquid/solid interfaces using resonant inelastic soft X-ray scattering (RIXS) and illustrate the value of the experimental approach with a few instructional examples. Using a high-transmission, high-resolution soft X-ray spectrometer, we are able to measure complete RIXS maps, i.e., record the soft X-ray emission intensity as a function of emission and absorption energy. As a first example, we show that a comparison of RIXS maps of “normal” and deuterated liquid and gas-phase water allows us to identify dissociation processes on the time scale of the oxygen 1 s core-hole lifetime. Similar dissociation effects are found for aqueous solutions of ammonia and amino acids. For the latter, the pH value has a strong influence on the nitrogen K emission spectra, which can thus be used to identify protonation and deprotonation processes in the solution. Finally, we review the investigation of the interface between liquid water and a CuIn(S,Se) 2 thin-film solar cell absorber, demonstrating the power of the technique to study liquid–solid interfaces in real-world systems. Under X-ray irradiation, the formation of sulfate on the absorber surface can be found." @default.
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- W2023996779 date "2013-06-01" @default.
- W2023996779 modified "2023-10-10" @default.
- W2023996779 title "RIXS investigations of liquids, solutions, and liquid/solid interfaces" @default.
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- W2023996779 doi "https://doi.org/10.1016/j.elspec.2012.10.006" @default.
- W2023996779 hasPublicationYear "2013" @default.
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