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• W2024003504 startingPage "10832" @default.
• W2024003504 abstract "Ionic and covalent combinations of oleic acid and Jeffamine ED900, a homoditopic polyetheramine, lead to novel porogens, either cataniomeric or nonionic surfactants, bearing respectively ammonium/carboxylate ionic pairs and/or amidic bonds. The effect of the electrostatic interaction vs. the covalent bond at the molecular level is clearly evidenced by the differences in the self-assembling behaviour, in either micellar or liquid crystal domains. Organized mesoporous materials were prepared through the cooperative templating mechanism from micelles and a silica source. The optimal reaction conditions were different for the nonionic (A) and di-ionic (B) surfactants, and the resulting materials had various morphologies (rod-like vs. spheres) and pore sizes (4 vs. 14 nm). Interestingly, the hybrid surfactant exhibits a versatile behaviour regarding the silica formation, acting as either a nonionic or a di-ionic surfactant in its respectively optimal conditions, A or B. This behaviour highlights the uniqueness of dynamic micelles as a novel supramolecular tool for the design of tailored mesoporous materials and could represent a novel platform for the design of pH responsive controlled drug delivery systems." @default.
• W2024003504 created "2016-06-24" @default.
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• W2024003504 date "2013-01-01" @default.
• W2024003504 modified "2023-10-09" @default.
• W2024003504 title "Electrostatic vs. covalent bond in modified Jeffamine: effect on the phase behaviour and on the templating of mesoporous silica" @default.
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• W2024003504 doi "https://doi.org/10.1039/c3sm52018h" @default.
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