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- W2024016072 abstract "The vibrational energy exchange between the stretching modes of H2O in the H2O + Ar collision has been studied in a semiclassical method in the temperature range of 200–3000 K. The energy exchange probability increases slowly, but nearly linearly, with temperature over the entire range, reflecting a near-resonant case. The intermolecular removal of the energy mismatch (ΔE = + 105 cm−1) by translation is found to be nearly as efficient as the intermolecular transfer to the rotational motion. The energy exchange probability for D2O + Ar is less efficiency by a factor of about two over the temperature range in both the intramolecular VR and intermolecular VT processes. The lower efficiency found in the VR step is due to a slower rotational motion of D2O, while that in the VT process is due to a larger energy mismatch for the D2O + Ar collision (ΔE = + 122 cm−1). The effect of molecular attraction is found to be important in the energy exchange process especially near room temperature, and the use of empirically determined attractive energies for the H2O—Ar complex is found to be valuable at such temperatures." @default.
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- W2024016072 title "Temperature dependence of the probability of vibrational energy exchange between the stretching modes in H2O/D2O + Ar collisions" @default.
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- W2024016072 doi "https://doi.org/10.1016/0009-2614(92)85658-w" @default.
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