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• W2024018422 startingPage "4598" @default.
• W2024018422 abstract "Time domain absorption spectroscopy using a tunable, infrared diode laser has been used to monitor the vibrational excitation of CO2 produced in the 193 nm excimer laser photolysis of gas phase pyruvic acid (CH3COCOOH). Nascent vibrational populations were measured in the following ten vibrational states of CO2: 0000, 0110, 0220, 0330, 0440, 0001, 0002, 0003, 0111, and 0221. Approximately 97% of the CO2 photoproduct is observed to be directly formed in the vibrational ground state. The remaining molecules are formed with a significant degree of vibrational excitation, having mode temperatures T(ν2)=1800±150 K, T(ν3)=3700 ±1000 K, T(ν2+ν3)=2000±400 K. The present experimental data suggest that the 193 nm photolysis may proceed through more than a single dissociation channel and involve a number of different photofragments." @default.
• W2024018422 created "2016-06-24" @default.
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• W2024018422 date "1987-10-15" @default.
• W2024018422 modified "2023-10-17" @default.
• W2024018422 title "IR diode laser study of vibrational energy distribution in CO2 produced by UV excimer laser photofragmentation of pyruvic acid" @default.
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• W2024018422 doi "https://doi.org/10.1063/1.453711" @default.
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