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- W2024018819 abstract "The edge effect function (expressing enhanced current due to diffusion across an edge) is determined for diffusion-limited, reversible, irreversible, and quasi-reversible forms of simple electron transfer following a potential step at a semi-infinite strip electrode. The derivation involves the application of Laplace and Fourier transforms and solution of the transformed problem by the Wiener–Hopf technique. The edge effect functions for the diffusion-limited, reversible, and irreversible cases are obtained explicitly; the Laplace transform of the edge effect function for the quasi-reversible case is obtained. The response of a planar electrode to a potential step can be viewed as a sum of (1) a contribution proportional to the area and immediately significant; (2) a contribution proportional to the perimeter and becoming significant over a longer time interval; (3) further contributions determined by more subtle geometric features and becoming significant at yet longer times. The area contribution is determined by the well-known shielded planar electrode model. The perimeter contribution is given by the results of this paper, which extend results for the diffusion-limited case first derived by Oldham [K.B. Oldham, J. Electroanal. Chem. 122 (1981), 1–17]." @default.
- W2024018819 created "2016-06-24" @default.
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- W2024018819 date "1997-12-01" @default.
- W2024018819 modified "2023-09-23" @default.
- W2024018819 title "The edge effect for planar electrodes" @default.
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- W2024018819 doi "https://doi.org/10.1016/s0022-0728(97)00367-7" @default.
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