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• W2024040585 abstract "The complexes trans-[Ru(CC-4-C6H4F)X(dppe)2] [X = Cl (1), CCPh (2), CC-4-C6H4NO2 (3)], trans-[Ru{CC-4-C6H4-(E)-CHCH-4-C6H4NO2}X(dppe)2] [X = CCPh (4), CC-4-C6H4CCPh (5)], and [C6H3-1,3-{CC-trans-[RuCl(dppe)2]}2-5-(CC-4-C6H4F)] (6) have been synthesized and the identity of 1 confirmed by a single-crystal X-ray diffraction study. Cyclic voltammetry reveals a metal-centered oxidation, the potential of which is largely invariant on alkynyl ligand replacement across the series 1–5; the diruthenium complex 6 shows two oxidation processes, consistent with weakly interacting metal centers. Hyper-Rayleigh scattering (HRS) studies at 1064 nm using ns pulses suggest quadratic nonlinearities for 3–5 that are amongst the largest thus far for organometallic complexes, a trend maintained with the two-level-corrected data. HRS studies at 800 nm using fs pulses and amplitude modulation to remove multi-photon fluorescence contributions reveal significant fluorescence-free nonlinearities for 3–5; the frequency-independent nonlinearities calculated from the 800 nm results are suggestive of fluorescence contributions to the 1064 nm data. Z-scan studies at 820 nm reveal cubic nonlinearities that increase with the size of the π-system, although error margins are significant." @default.
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• W2024040585 date "2006-02-01" @default.
• W2024040585 modified "2023-10-17" @default.
• W2024040585 title "Organometallic complexes for nonlinear optics. Part 36. Quadratic and cubic optical nonlinearities of 4-fluorophenylethynyl- and 4-nitro-(E)-stilbenylethynylruthenium complexes" @default.
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• W2024040585 doi "https://doi.org/10.1016/j.ica.2005.09.012" @default.
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