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- W2024106345 abstract "V-R.T and V-V processes in methane-inert-gas mixtures are studied optoacoustically following excitation of the CH4 ν3 level with a HeNe laser at 2947.9 cm−1. The dominant route of deactivation, after fast equilibration of levels ν3 and ν1. is (ν3. ν1) → 2ν4 → ν4 + ν4: the bending modes ν4 and ν2 then come to equilibrium and rela??? to the rotational, translational modes. Rate constants are reported with inert gases He, Ne and Xe, for (a) (ν3. ν1) → 2ν4. (b) ν2 → ν4 and (c) the single-quantum step (ν3. ν1) → (ν2. ν4). In addition the intermolecular process in CH4 collisions. 2ν4 → ν4 + ν4. is shown to have a rate constant of 1.0±0.25 ns−1 atm−1." @default.
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- W2024106345 date "1983-01-01" @default.
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- W2024106345 title "Vibrational-translational/rotational and vibrational-vibrational processes in methane/inert-gas mixtures: Optoacoustic phase measurements" @default.
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- W2024106345 doi "https://doi.org/10.1016/0301-0104(83)80004-4" @default.
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