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- W2024124676 abstract "Abstract A key challenge in processing carbon nanotubes and their composites for large‐scale applications is aggregation. Cation–π stacking interactions have been discovered to disperse heavily entangled single‐walled carbon nanotube (SWNT) bundles in ionic liquids (ILs). In this work, we found that a dispersible, silky single‐layer graphene (SLG) can be readily gathered together to form a crosslinked gel after entrapping sufficient IL molecular via the likely noncovalent interaction. By incorporating the dispersed SWNTs into the gathered SLG gel synchronously, we prepared solid, finely crosslinked SWNTs–SLG films, assisted by an avenue of 2‐step extraction to remove the IL completely. The gel‐derived SWNTs–SLG complex film was applied as a support material of oxygen cathodes for Li–O 2 batteries. It exhibited a remarkable improved cycleability in comparison to made of SWNTs and SLG alone due to the finely crosslinked feature. Decorated SWNTs and SLG can also form gel‐derived complexes via the same process to construct support–catalyst complexes. A SWNTs–SLG film loaded with Ru nanoparticles exhibited not only catalytic effects, but also the ability to suppress the side reactions, and hence stabilized the whole Li–O 2 battery. Our research introduces a gel‐derived, high‐dispersed processing of carbon nanotube‐graphene complexes and demonstrates their favorable applications on Li–O 2 batteries." @default.
- W2024124676 created "2016-06-24" @default.
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- W2024124676 date "2014-08-27" @default.
- W2024124676 modified "2023-10-18" @default.
- W2024124676 title "Gel-Derived Cation-π Stacking Films of Carbon Nanotube-Graphene Complexes as Oxygen Cathodes" @default.
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- W2024124676 doi "https://doi.org/10.1002/cssc.201402567" @default.
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