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- W2024190875 abstract "Based on experimental evidence for the adsorbate-induced hex → 1 × 1 transformation of the Pt(100) surface structure the following model is proposed: The 20% surplus atoms segregate on top of the 1 × 1 plane, where they migrate and may form islands whose average size varies with temperature. This process is computer simulated by means of the Monte Carlo technique, with ϵ = VkBT, the (attractive) pairwise interaction energy between neighbouring adparticles divided by kBT being an adjustable parameter. Only in a relatively narrow range of ϵ (about − 3 to −4) large islands may develop; for low values of ϵ (high T) the island size distribution is thermodynamically limited and is characterized by a large fraction of isolated adatoms, while at high ϵ (low T) kinetic limitations prevent the formation of larger islands. Qualitative agreement with experimental data is obtained with V estimated to be about −20 kJmol." @default.
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- W2024190875 date "1989-08-01" @default.
- W2024190875 modified "2023-10-16" @default.
- W2024190875 title "Computer simulations of the adsorbate-induced structural transformation of Pt(100)" @default.
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- W2024190875 doi "https://doi.org/10.1016/0039-6028(89)90162-3" @default.
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