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• W2024203764 startingPage "6594" @default.
• W2024203764 abstract "${mathrm{YBa}}_{2}$${mathrm{Cu}}_{3}$${mathrm{O}}_{6+mathrm{x}}$ is known to undergo a transition from a magnetic semiconductor to a metallic high-temperature superconductor as the oxygen content is increased from the range 0.0ensuremath{le}xensuremath{le}0.5 to 0.5ensuremath{le}xensuremath{le}1.0. We report here detailed temperature-dependent magnetic-susceptibility studies for x in the composition range 0.0ensuremath{le}xensuremath{le}1.0. For 0.05ensuremath{le}xensuremath{le}0.5, the effective moment ${ensuremath{mu}}_{mathrm{eff}}$ decreases with decreasing temperature from 300--160 K, as expected for an antiferromagnet whose N'eel temperature is above room temperature. Below 160 K, ${ensuremath{mu}}_{mathrm{eff}}$ increases, reaching a maximum at ensuremath{sim}40 K then decreases again. The magnitude of this low-temperature peak in ${ensuremath{mu}}_{mathrm{eff}}$ increases with x, reaches a maximum at x=0.35, then decreases toward zero. A Monte Carlo simulation method has been used to model the three-dimensional antiferromagnetic ordering of this system as a function of oxygen composition. The calculation reveals the presence of spin frustration as x increases from 0 to 0.3 in accord with the increasing number of effective moments at low temperatures. Above x=0.3 a new long-range order (corresponding to a doubling of the magnetic unit cell perpendicular to the planes) is predicted to occur in agreement with the observed magnetic susceptibility and recent neutron-diffraction experiments of Kadowaki et al. and Lynn et al. Above x=0.5, relatively few localized moments are observed in the temperature-dependent susceptibility measurement. In the metallic regime the ``Pauli susceptibility'' is observed to increase approximately linearly with oxygen content. This is in accord with decreasing effects of antiferromagnetic correlation with increasing x." @default.
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• W2024203764 date "1989-04-01" @default.
• W2024203764 modified "2023-09-23" @default.
• W2024203764 title "Magnetic susceptibility ofYBa2Cu3O6+x: Effects of spin frustration and correlation" @default.
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• W2024203764 doi "https://doi.org/10.1103/physrevb.39.6594" @default.
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