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- W2024280006 abstract "n -Butanethiol-impregnated, micrometric, pristine Ni powder (Ni–C 4 S) was tested as a catalyst for use in the steam reforming of methane, using X-Ray photoemission spectroscopy (XPS) and mass spectrometry (MS). The catalytic activities of both the pristine Ni and the Ni–C 4 S powders were measured at 700 °C, under conditions that favoured (molar CH 4 :H 2 O ratio of 2:1), and did not favour (molar CH 4 :H 2 O ratio of 1:2) formation of surface carbon. The results show that: (a) Ni–C 4 S demonstrates both high catalytic activity and stability during the 21 h duration test; (b) under conditions favouring the deposition of surface carbon, the Ni–C 4 S retained both its efficiency and structural integrity, while the catalytic activity of the Ni was reduced by ∼70% and the catalyst pellets lost their integrity; (c) the amount of deposited carbon in the case of the Ni–C 4 S catalyst was significantly lower than that observed for the Ni catalyst, in spite of the longer testing duration. It was concluded that the thiols pre-treatment of Ni surfaces, to be subsequently used in the production of catalysts supported SOFC anodes, can considerably increase their “active life span” this being a critical attribute in respect of their eventual commercialization." @default.
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- W2024280006 date "2007-09-01" @default.
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- W2024280006 title "Inhibition of carbon formation during steam reforming of methane using thiol-coated nickel catalysts" @default.
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- W2024280006 doi "https://doi.org/10.1016/j.jpowsour.2007.07.016" @default.
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