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• W2024287270 endingPage "1918" @default.
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• W2024287270 abstract "Product selectivity and yields of cyclohexanol and cyclohexanone formation in the photocatalytic air oxidation of cyclohexane on TiO(2) particles were determined as a function of the irradiation wavelength (254 < or = lambda/nm < or = 366) and the photon flux (0.3 < or = I(0)/neinstein cm(-2) s(-1) < or = 5.0). Photonic efficiencies for total monooxygenated products (cyclohexanol + cyclohexanone) ranged from 10 to 25% depending on photon energy and fluency. The cyclohexanol-to-cyclohexanone ratio linearly increases with the incident photon flux at each wavelength and varies more than a magnitude order -- from 3 to 32%-at the same incident photon fluency -- 5 neinstein cm(-2) s(-1) -- by changing the irradiation wavelength from 366 to 303 nm. Experimental evidence indicates that both spectral and intensity effects emerge as a consequence of the change in the frequency of photon absorption per particle. A mechanism is proposed which accounts for the origin of the selectivity changes." @default.
• W2024287270 created "2016-06-24" @default.
• W2024287270 creator A5004574855 @default.
• W2024287270 creator A5054624105 @default.
• W2024287270 date "2005-01-19" @default.
• W2024287270 modified "2023-10-18" @default.
• W2024287270 title "Photon Flux and Wavelength Effects on the Selectivity and Product Yields of the Photocatalytic Air Oxidation of Neat Cyclohexane on TiO₂ Particles" @default.
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• W2024287270 doi "https://doi.org/10.1021/jp045602+" @default.
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