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• W2024332937 endingPage "4226" @default.
• W2024332937 startingPage "4215" @default.
• W2024332937 abstract "The study of Al speciation is of interest for the assessment of soil and water quality. For the measurement of free aluminum (Al3+), a recently developed Donnan membrane technique was tested by measuring Al3+ in aluminum-fluoride solutions and gibbsite suspensions. It shows that the Donnan membrane technique can measure free Al3+ reliably up to 10(-9) M and the equilibration takes 3-4 days. Next, Al binding to humic acid (HA) purified from a forest soil was measured using either the Donnan membrane technique or gibbsite suspension. Results were compared with those predicted with the non-ideal consistent competitive adsorption (NICA)-Donnan model. The predictions using the generic parameters without fitting were in reasonable agreement with the measured data. Finally, the Donnan membrane technique was used to determine Al binding to dissolved organic matter (DOM) in the solutions of 24 soil samples at pH interval of 3-7. Measurements agree well with the predictions using the NICA-Donnan model assuming 30% of DOM is HA and 30% is fulvic acid. With this model, the effects of pH and DOM changes on the concentration of Al in 81 soil solutions were predicted reasonably without adjustment of model parameters. The comparison between the results of analysis and the modeling provides a mutual validation for the two methods." @default.
• W2024332937 created "2016-06-24" @default.
• W2024332937 creator A5023230008 @default.
• W2024332937 creator A5038953308 @default.
• W2024332937 creator A5062759057 @default.
• W2024332937 date "2002-10-01" @default.
• W2024332937 modified "2023-10-14" @default.
• W2024332937 title "Aluminum speciation in natural waters: measurement using Donnan membrane technique and modeling using NICA-Donnan" @default.
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• W2024332937 doi "https://doi.org/10.1016/s0043-1354(02)00166-5" @default.
• W2024332937 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/12420926" @default.
• W2024332937 hasPublicationYear "2002" @default.
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