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- W2024346757 abstract "We present a detailed study of the photoinduced insulator-metal transition in VO${}_{2}$ with broadband time-resolved reflection spectroscopy. This allows us to separate the response of the lattice vibrations from the electronic dynamics and observe their individual evolution. When we excite VO${}_{2}$ above the photoinduced phase transition threshold, we find that the restoring forces that describe the ground-state monoclinic structure are lost during the excitation process, suggesting that an ultrafast change in the lattice potential drives the structural transition. However, by performing a series of pump-probe measurements during the nonequilibrium transition, we observe that the electronic properties of the material evolve on a different, slower time scale. This separation of time scales suggests that the early state of VO${}_{2}$, immediately after photoexcitation, is a nonequilibrium state that is not well defined by either the insulating or the metallic phase." @default.
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- W2024346757 date "2013-03-20" @default.
- W2024346757 modified "2023-10-09" @default.
- W2024346757 title "Tracking the evolution of electronic and structural properties of VO<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:msub><mml:mrow /><mml:mn>2</mml:mn></mml:msub></mml:math>during the ultrafast photoinduced insulator-metal transition" @default.
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- W2024346757 doi "https://doi.org/10.1103/physrevb.87.115126" @default.
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