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- W2024351433 abstract "Tautomerism of the nucleobase uracil is characterized in the gas phase through IR photodissociation spectroscopy of singly hydrated protonated uracil created with tandem mass spectrometric methods in a commercially available Fourier transform ion cyclotron resonance mass spectrometer. Protonated uracil ions generated by electrospray ionization are re-solvated in a low-pressure collision cell filled with a mixture of water vapor seeded in argon. Their structure is investigated by IR photodissociation spectroscopy in the NH and OH stretching region (2500−3800 cm−1) with a tabletop IR laser source and in the 1000−2000 cm−1 range with a free-electron laser. In both regions the IR photodissociation spectrum exhibits well-resolved spectral signatures that point to the presence of two different types of structure for monohydrated protonated uracil, which result from the two lowest-energy tautomers of uracil. Ab initio calculations confirm that no water-catalyzed tautomerization occurs during the re-solvation process, indicating that the two protonated forms of uracil directly originate from the electrospray process." @default.
- W2024351433 created "2016-06-24" @default.
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- W2024351433 date "2008-11-11" @default.
- W2024351433 modified "2023-10-17" @default.
- W2024351433 title "Tautomerism of Uracil Probed via Infrared Spectroscopy of Singly Hydrated Protonated Uracil" @default.
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- W2024351433 doi "https://doi.org/10.1021/jp806396t" @default.
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