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- W2024414164 abstract "A possible experimental explanation for the unusual temperature dependence of water line broadening by molecular hydrogen recently observed by Dick et al. [Phys. Rev. A 81, 022706 (2010)] is proposed. This temperature dependence differs radically from both theoretical predictions and the higher temperature behavior, but remains unexplained. It is suggested that the cause is a change in sample composition due to preferential adsorption of orthohydrogen onto the cell walls at low temperature. As parahydrogen has collision cross sections with water molecules up to an order of magnitude smaller than those with orthohydrogen, an enrichment of the gas sample by parahydrogen would lead to a decrease in broadening parameters at low temperatures, as observed in the experiment." @default.
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- W2024414164 date "2010-09-29" @default.
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- W2024414164 title "Comment on “Collisional cooling investigation of THz rotational transitions of water”" @default.
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- W2024414164 doi "https://doi.org/10.1103/physreva.82.036703" @default.
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