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• W2024449326 startingPage "5079" @default.
• W2024449326 abstract "Readily available chiral primary 1,2-aminoalcohols and diamines have been explored as organocatalysts for a domino Michael–aldol reaction. Their application in this organocascade process afforded cyclohexanone A with high levels of reactivity (up to 91% yield) and stereoselectivity (>97 : 3 d.r., up to 93% ee). Depending on the acid cocatalyst different chiral species (cyclic secondary aminesvs. acyclic primary amines) might catalyse the process. In order to shed light on the catalytic activation, several experiments were carried out and a detailed possible reaction mechanism is proposed. Theoretical studies support the stereochemical outcome of the process." @default.
• W2024449326 created "2016-06-24" @default.
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• W2024449326 date "2011-01-01" @default.
• W2024449326 modified "2023-10-06" @default.
• W2024449326 title "First asymmetric cascade reaction catalysed by chiral primary aminoalcohols" @default.
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• W2024449326 doi "https://doi.org/10.1039/c1ob05400g" @default.
• W2024449326 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/21614385" @default.
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