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- W2024480670 abstract "Theoretical relations have been derived for the electrochemical monitoring of a second-order decay of radicals generated by flash photolysis or pulse radiolysis, taking into account the inhomogeneous decay-rate profile in the diffusion layer. The derivations are given for the planar electrode, the stationary sphere (e.g. hanging drop) and the “expanding plane” model of the dropping mercury electrode (DME) as well as for the DME including spherical diffusion. It is shown that the approximation proposed by Birk and Perone3 would result in a consistent error of 27% of the rate constant, and that additional modifications are necessary for electrodes other than the stationary plane. Recommendations are given for practical application for the types of electrodes mentioned above." @default.
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- W2024480670 date "1974-10-01" @default.
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- W2024480670 title "On the electrochemical observation of a second-order decay of radicals generated by flash photolysis or pulse radiolysis" @default.
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