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• W2024558802 abstract "Abstract In this paper we report fluorescence excitation and dispersed emission of the aniline-benzene van der Waals complex formed in a supersonic expansion. The excitation spectrum of the complex which shows well structured progressions is red shifted by about 450 cm−1 relative to the origin of aniline which implies that the excited state is more strongly bound than the ground state. The fluorescence spectra appear to be composed of broad overlapping bands attributed to transitions from the excited states involving large and displaced Franck-Condon distributions and fast redistribution. Experimental observations are supported by empirical calculations using Buckingham potentials based on atom-atom interactions. Optimization of the geometry leads to favored face geometry of both aromatic rings, with the excited state being more strongly bound than the ground state as it was observed experimentally. Calculated vibrational modes and Franck-Condon distributions lead us to assign the main vibrational structure in the excited state to slipping motion along the symmetry axis of the complex." @default.
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• W2024558802 date "1988-02-01" @default.
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• W2024558802 title "Molecular jet study and calculations of the vibronic structure of the aniline-benzene van der Waals complex" @default.
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• W2024558802 doi "https://doi.org/10.1016/0301-0104(88)87167-2" @default.
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