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• W2024568033 abstract "YbCu6.5 with hexagonal CaCu5-type structure was found to exhibit enhanced Pauli paramagnetism (∼10−3 emu/mole) with a broad maximum in its susceptibility–temperature curve at ∼1000 K for the first time. The Cu/Al substitution causes the maximum to shift systematically towards lower temperature and to disappear at x=1. Meanwhile the magnitude of susceptibility increases continuously. For x≥1.5, Curie–Weiss behavior is established with an effective magnetic moment Peff close to 4.54 μB of free Yb3+ ion. Al substitution therefore drives the Yb ion from a nearly divalent state for x=0, via a strongly mixed-valence states for 0<x<1.5, to a stable localized trivalent state for 1.5≤x≤2. As a substantial evidence for the Yb intermediate valent state, an anomalous lattice contraction is observed as the Al content increases from x=1 to x=0.5." @default.
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• W2024568033 date "2001-07-01" @default.
• W2024568033 modified "2023-09-23" @default.
• W2024568033 title "Magnetic properties of hexagonal YbCu5−xAlx" @default.
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• W2024568033 doi "https://doi.org/10.1016/s0925-8388(01)01385-8" @default.
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