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• W2024600314 endingPage "3974" @default.
• W2024600314 startingPage "3974" @default.
• W2024600314 abstract "Four new Ni(II) coordination polymers containing dipyridyl amide and angular dicarboxylate ligands, {[Ni(L1)(MBA)]·2H2O}∞ [L1 = N,N′-di(4-pyridyl)-adipoamide; H2MBA = diphenylmethane-4,4′-dicarboxylic acid], 1, {[Ni(L1)(OBA)]·H2O}∞ [H2OBA = 4,4′-oxybis(benzoic acid)], 2, {[Ni(L1)(SDA)]·2H2O}∞ (H2SDA = 4,4′-sulfonyldibenzoic acid), 3, and {[Ni2(L2)(SDA)2]·6H2O}∞ [L2 = N,N′-di(4-pyridyl)suberoamide], 4, have been synthesized by hydrothermal reactions and were structurally characterized by single crystal X-ray diffraction analyses. Complex 1 is a 1D → 2D polycatenane derived from the helical channels, and the 2D layers are further mutually interdigitated, whereas complex 2 forms 2D rhombic grids with the (6,4) topology, which are interwoven with each other to give a two fold 2D → 2D interpenetrating net. Complex 3 shows the 1D looped chain structure, and complex 4 shows 2D layers which catenate to each other to form a 2D → 3D inclined polycatenation framework with the new (42·68·8·104)(4)2 topology. The C–X–C (X = CH2, 1; O, 2; and SO2, 3 and 4) angles are important in determining the structural diversity. Complex 1 exhibits a different magnetic reaction in the ZFC and FC processes, revealing the existence of a meta-state of ferromagnetic ordering, whereas the activation energies of spin–orbit coupling and antiferromagnetic interaction of complexes 2–4 are directed by the N⋯N and Ni⋯Ni distances, respectively." @default.
• W2024600314 created "2016-06-24" @default.
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• W2024600314 date "2013-01-01" @default.
• W2024600314 modified "2023-09-30" @default.
• W2024600314 title "Structural diversity of Ni(ii) coordination polymers containing dipyridyl amide and angular dicarboxylate ligands: synthesis, structures and magnetism" @default.
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• W2024600314 doi "https://doi.org/10.1039/c3ce26928k" @default.
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