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- W2024646303 abstract "Calorimetric measurements on K${mathrm{D}}_{2}$P${mathrm{O}}_{4}$ have been conducted, and the transition is found to be first order with an entropy change at ${T}_{c}$ of $(0.2407ifmmodepmelsetextpmfi{}0.0016)R$. The entropy change associated with destruction of the polarization from 0ifmmode^circelsetextdegreefi{}K to ${T}_{c}$ is found to be $(0.4234ifmmodepmelsetextpmfi{}0.0071)R$. It is shown that a mean-field theory of the type proposed by Silsbee, Uehling, and Schmidt can give a good account of the heat capacity and polarization to within about 1ifmmode^circelsetextdegreefi{}K of ${T}_{c}$, although the latent heat and entropy are not predicted satisfactorily, presumably because of the breakdown of the mean-field approximation close to the transition. Below ${T}_{c}$ the divergence in the heat capacity may be argued to be logarithmic in the region closer than 1ifmmode^circelsetextdegreefi{} to ${T}_{c}$, or to be as $frac{1}{{({T}_{c}ensuremath{-}T)}^{frac{1}{2}}}$ in the region ${T}_{c}ensuremath{-}2ifmmode^circelsetextdegreefi{}<T<{T}_{c}ensuremath{-}0.2ifmmode^circelsetextdegreefi{}$. Arguments are offered in favor of the logarithmic divergence." @default.
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- W2024646303 date "1968-03-10" @default.
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- W2024646303 title "Studies of Phase Transitions in Order-Disorder Ferroelectrics. II. Calorimetric Investigations of KD2PO4" @default.
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- W2024646303 doi "https://doi.org/10.1103/physrev.167.504" @default.
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