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• W2024650041 startingPage "1007" @default.
• W2024650041 abstract "The rate of vibrational energy relaxation (VER) is a valuable probe of microscopic intermolecular interaction. In the present article, the VER rate of the T1u CO stretch of W(CO)6 is measured in binary solutions composed of an alkane (hexane, decane, tetradecane) and cyclohexane or CCl4, with seven mixing volume ratios. The volume ratio dependence indicates that, among the three alkane−cyclohexane solutions, only decane shows an exceptionally strong contribution to the VER process. It is strongly suggested that decane forms a specific solute−solvent complex with W(CO)6. The “V-shaped” dependence of the VER rate on the number of carbons in alkane solvents (Banno, M.; Sato, S.; Iwata, K.; Hamaguchi, H. Chem. Phys. Lett. 2005, 412, 464.) is explained by the solute−solvent complex model. There are no experimental results that suggest the formation of the specific solute−solvent complex in alkane−CCl4 solutions." @default.
• W2024650041 created "2016-06-24" @default.
• W2024650041 creator A5034929812 @default.
• W2024650041 creator A5036589908 @default.
• W2024650041 creator A5045212371 @default.
• W2024650041 date "2009-01-08" @default.
• W2024650041 modified "2023-10-03" @default.
• W2024650041 title "Intermolecular Interaction between W(CO)₆ and Alkane Molecules Probed by Ultrafast Vibrational Energy Relaxation: Anomalously Strong Interaction between W(CO)₆ and Decane" @default.
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• W2024650041 doi "https://doi.org/10.1021/jp805518d" @default.
• W2024650041 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/19193172" @default.
• W2024650041 hasPublicationYear "2009" @default.
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