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- W2024653075 abstract "The increasing importance of heat transformation applications of adsorption (refrigeration, heat pumping, and heat storage) creates a demand for adsorbents optimized in new ways. The figures of merit in these applications are different from those that guide most adsorbent design processes today. A quantity to be optimized is the total sorptive heat stored over a cycle period rather than selectivity or total adsorption capacity. This optimization requires a detailed understanding of the link between cycle thermodynamics and microscopic adsorbent characteristics. We show that a simple statistical Langmuir model of adsorption is sufficient to analyze some of the key relationships. The influence of energetic heterogeneity on cycle performance is analyzed in a model system in relation to the energy and entropy change upon adsorption. For a homogeneous system of monoenergetic adsorption sites, it is shown that for each value of the adsorbed state entropy there is an optimal adsorbent−adsorbate interaction energ..." @default.
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- W2024653075 date "2003-09-04" @default.
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- W2024653075 title "Influence of Adsorbent Characteristics on the Performance of an Adsorption Heat Storage Cycle" @default.
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- W2024653075 doi "https://doi.org/10.1021/ie0300169" @default.
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