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• W2024653881 endingPage "1684" @default.
• W2024653881 startingPage "1676" @default.
• W2024653881 abstract "Ru nanoclusters self-assemble over macroscopic sample areas during vapor deposition of Ru on monolayer graphene (MLG) on Ru(0001). The Ru nanoclusters form arrays with a mean lateral cluster diameter of ~ 20 Å, cluster heights of 1 or 2 ML, and a size distribution that remains nearly constant with increasing coverage. Combined scanning tunneling microscopy and density functional theory (DFT) show that the clusters are templated by the MLG/Ru(0001) moiré unit cell and identify the preferred binding site of the clusters as the low fcc region of the moiré. Cross-sectional transmission electron microscopy (TEM) and high-resolution TEM contrast simulations experimentally demonstrate that the interaction of the Ru clusters with the underlying MLG/Ru(0001) leads to a local lifting of the graphene layer of the template. DFT calculations confirm this mechanism of interaction of the Ru clusters with the strongly coupled MLG/Ru(0001). Weakening of the graphene-support coupling via oxygen intercalation is shown to have a major effect on the assembly of Ru nanocluster arrays. With a preferred binding site lacking on decoupled graphene, the Ru nanoclusters grow significantly larger, and clusters with 1 to 4 ML height can coexist." @default.
• W2024653881 created "2016-06-24" @default.
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• W2024653881 date "2011-09-01" @default.
• W2024653881 modified "2023-09-25" @default.
• W2024653881 title "Arrays of Ru nanoclusters with narrow size distribution templated by monolayer graphene on Ru" @default.
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• W2024653881 doi "https://doi.org/10.1016/j.susc.2011.01.026" @default.
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