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- W2024703695 abstract "This chapter presents an overview on the implication of microporous zeolites and ordered mesoporous silica-based materials in electrochemistry. There are numerous reasons why zeolites and mesoporous silicates are attractive for electrochemical applications. Zeolites constitute a unique family of materials displaying both ion exchange capacity and size selectivity in a single component. This would impart both charge and size selectivity properties. The most commonly used zeolites in connection to electrochemistry are those characterized by a rather high ion exchange capacity, such as zeolites A, X, Y, L, mordenite, among some others. Silica-based materials, and especially organic-inorganic hybrids, exhibit chemical and physico-chemical features that might be readily exploited when used to modify electrode surfaces. The electrochemical responses of ZMEs prepared with zeolite particles previously loaded with redox species have been widely studied in order to understand why such species located in an insulating environment are likely to undergo charge-transfer reactions and how the microporous host would affect their electrochemical behavior. Most electron transfer reactions involved associated mass transport so that diffusion processes often limited the sensitivity of the devices. Advanced applications of electrodes modified with microporous zeolites and ordered mesoporous (organo)silica materials were mostly developed in the field of electroanalysis. Some other applications involving zeolites and MPS in electrochemistry have been reported, including gas sensors, potentiometry, electrochemiluminescence, and photoelectrochemistry. MPS films deposited on electrode surfaces are sensitive to gas adsorption, resulting in measurable conductivity changes that can be exploited to detect gaseous analytes. Zeolite-polymer composite membranes as well as binder-free zeolite membranes have been prepared for applications in potentiometric sensing." @default.
- W2024703695 created "2016-06-24" @default.
- W2024703695 creator A5089514392 @default.
- W2024703695 date "2009-01-01" @default.
- W2024703695 modified "2023-09-25" @default.
- W2024703695 title "Electrochemistry with Micro- and Mesoporous Silicates" @default.
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