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• W2024762347 abstract "${mathrm{NdBaCo}}_{2}{mathrm{O}}_{5.47}$ cobaltite has been investigated using neutron and synchrotron powder diffraction. At ${T}_{mathrm{MI}}ensuremath{sim}360mathrm{K},$ the compound exhibits an associated metal-insulator and spin-state transition commonly observed in these systems. At ${T}_{N}ensuremath{sim}275mathrm{K},$ the $mathrm{IS}ensuremath{-}{mathrm{Co}}^{3+}$ species order in a AFM G-type structure. At ${T}_{mathrm{SSO}}ensuremath{sim}230mathrm{K},$ the AFM G-type volume fraction is gradually transformed into spin-state ordered clusters having a distinct magnetic structure. These clusters result from a selective $mathrm{IS}ensuremath{-}{mathrm{Co}}^{3+}$ ${(t}_{2g}^{5}{e}_{g}^{1})$ to $mathrm{LS}ensuremath{-}{mathrm{Co}}^{mathrm{III}}$ ${(t}_{2g}^{6}{e}_{g}^{0})$ crossover and the ordering of the diamagnetic ions over $ensuremath{sim}350mathrm{AA{}}$ correlation lengths. The same electronic phase segregation is observed in ${mathrm{TbBaCo}}_{2}{mathrm{O}}_{5.46}$ and seems to occur only for a narrow range of oxygen stoichiometry." @default.
• W2024762347 created "2016-06-24" @default.
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• W2024762347 date "2002-11-19" @default.
• W2024762347 modified "2023-10-13" @default.
• W2024762347 title "Spin-state ordered clusters in the perovskite<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant=normal>NdBaCo</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant=normal>O</mml:mi></mml:mrow><mml:mrow><mml:mn>5.47</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math>" @default.
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• W2024762347 doi "https://doi.org/10.1103/physrevb.66.184421" @default.
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