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- W2024862290 abstract "Metal organic coordination polymers (CPs), as most attractive multifunctional materials, have been studied extensively in many fields. However, metal-biomolecule CPs and CPs' electrochemical properties and applications were studied much less. We focus on this topic aiming at electrochemical biosensors with excellent performance and high biocompatibility. A new nanoscaled metal-biomolecule CP, Mn-tyr, containing manganese and tyrosine, was synthesized hydrothermally and characterized by various techniques, including XRD, TEM, EDS, EDX mapping, elemental analysis, XPS, and IR. Electrode modified with Mn-tyr showed novel bidirectional electrocatalytic ability toward both reduction and oxidation of H2O2, which might be due to Mn. With the assistance of CNTs, the sensing performance of Mn-tyr/CNTs/GCE was improved to a much higher level, with high sensitivity of 543 mA mol(-1) L cm(-2) in linear range of 1.00×10(-6)-1.02×10(-4) mol L(-1), and detection limit of 3.8×10(-7) mol L(-1). Mn-tyr/CNTs/GCE also showed fast response, high selectivity, high steadiness and reproducibility. The excellent performance implies that the metal-biomolecule CPs are promising candidates for using in enzyme-free electrochemical biosensing." @default.
- W2024862290 created "2016-06-24" @default.
- W2024862290 creator A5013926095 @default.
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- W2024862290 date "2015-05-01" @default.
- W2024862290 modified "2023-10-03" @default.
- W2024862290 title "Nanorods of a new metal–biomolecule coordination polymer showing novel bidirectional electrocatalytic activity and excellent performance in electrochemical sensing" @default.
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- W2024862290 doi "https://doi.org/10.1016/j.bios.2014.06.047" @default.
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