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- W2024862395 abstract "Infrared spectra of N2O trimers are studied using a tunable diode laser to probe a pulsed supersonic slit-jet expansion. A previous observation by Miller and Pedersen [J. Chem. Phys. 108, 436 (1998)] in the N2O ν1+ν3 combination band region (∼3480 cm−1) showed the trimer structure to be noncyclic, with three inequivalent N2O monomer units which could be thought of as an N2O dimer (slipped antiparallel configuration) plus a third monomer unit lying above the dimer plane. The present observations cover the N2O fundamental band regions ν3 (∼1280 cm−1) and ν1 (∼2230 cm−1). In the ν3 region, two trimer bands are assigned with vibrational shifts and other characteristics similar to those in the ν1+ν3 region, but in the ν1 region all three possible trimer bands are observed. Relationships among the various bands are considered with reference to their rotational intensity patterns, their vibrational shifts, and the properties of the related N2O dimer, with results that generally support the conclusions of Miller and Pedersen. Three trimer bands are also observed for the fully N15-substituted species in the ν1 region, and these results should aid in the detection of the as-yet-unobserved pure rotational microwave spectrum of the trimer." @default.
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- W2024862395 date "2009-01-23" @default.
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- W2024862395 title "New infrared spectra of the nitrous oxide trimer" @default.
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- W2024862395 doi "https://doi.org/10.1063/1.3062957" @default.
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