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- W2024872557 abstract "By the standard perturbation technique of Zimm, the second virial coefficient A2 is calculated in the ``double-contact'' approximation for mixtures of two polymers in a single solvent. The two solute molecules are alike chemically, but they differ in size (molecular weight) and/or geometry (in the sense of straight-chain, branched, or closed-ring architecture). From investigation of a number of pairs of species, some tentative generalizations emerge on limiting behavior for A2 small but positive, i.e., near, but above, the theta temperature. If the two polymer molecules have exactly the same structure and differ only in size (e.g., two straight chains of different molecular weight, two ring molecules of different weight), the virial coefficient, as measured by either osmotic pressure or light scattering, is always a monotone function of the proportions of the two components in the mixed solute; but when the models are different, there can exist a range of relative molecular weights of the two solutes within which A2 passes through a maximum as a function of composition. A minimum is never found." @default.
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- W2024872557 date "1966-10-15" @default.
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- W2024872557 title "Statistical Thermodynamics of Polymer Solutions. V. Interactions between Geometrically Dissimilar Polymer Chains in a Poor Solvent" @default.
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