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• W2024921297 abstract "The photodissociation dynamics of CBrCl3 was studied near 234 and 265 nm using a two-dimensional photofragment ion imaging technique. Bromine fragments monitored in this study were produced via direct dissociation of CBrCl3, represented by CBrCl3→CCl3+Br(2P1/2)/Br(2P3/2). The branching ratio of Br(2P1/2) (denoted Br*)/Br(2P3/2) (denoted Br) showed strong excitation energy dependence. The product quantum yields at two different excitation wavelengths were Φ 234 nm(Br*)=0.31±0.01 and Φ 265 nm(Br*)=0.68±0.02, respectively. The speed and angular distributions of Br* and Br fragments were determined. Similar values of β(234 nm)=−0.44 and β(265 nm)=−0.47 for Br were observed, while β values for Br* were found to be markedly different, β(234 nm)=−0.34 and β(265 nm)=1.43. The strong curve crossing, 1Q1→3Q0, and the angular distribution of Br* suggesting a typical perpendicular transition, were observed at 234 nm photodissociation." @default.
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• W2024921297 date "1999-09-01" @default.
• W2024921297 modified "2023-10-16" @default.
• W2024921297 title "Photodissociation of CBrCl3 at 234 and 265 nm: Evidence of the curve crossing" @default.
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• W2024921297 doi "https://doi.org/10.1063/1.479182" @default.
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