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- W2024922718 abstract "Reflection, time-integrated and time-resolved luminescence spectra have been measured in PbI 2(1-x) Br 2x (x≥0.5) mixed crystals in order to elucidate the excitonic properties and relaxation processes of orthorhombic phase PbI 2 embedded in the mixed crystals. The crystal structure of PbI 2(1-x) Br 2x above x=0.5 is orthorhombic and an observed new reflection peak (~2.5 × 10 4 cm -1 ) above x=0.5 is due to an excitonic state of orthorhombic phase PbI 2 . On the excitation energy above 2.5 × 10 4 cm -1 , a broad luminescence band with a large Stokes shift from the reflection peak was observed. This luminescence band is attributed to a self-trapped exciton state. The decay of the luminescence has two components. Based on an atomic excitation picture, the shorter decay component (≤10 ns ) is attributed to the allowed transition from 3 P 1 to 1 S 0 . On the other hand, the longer decay component (~3 μ s ) might be due to the forbidden transition from 3 P 0 to 1 S 0 ." @default.
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- W2024922718 date "2001-12-10" @default.
- W2024922718 modified "2023-09-27" @default.
- W2024922718 title "EXCITON DYNAMICS OF ORTHORHOMBIC PHASE PbI2 EMBEDDED IN PbI2-PbBr2 MIXED CRYSTALS" @default.
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- W2024922718 doi "https://doi.org/10.1142/s0217979201008810" @default.
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