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- W2024953935 abstract "We present results of calculations of the lifetimes of excited electrons (holes) in quantum well states and quantum well resonances in Pb overlayers supported on Cu(111). Many-body decay via inelastic energy relaxation and one-electron decay via energy-conserving one-electron transfer into the substrate are considered. One-electron energies and wave functions have been computed for different coverages of the Pb overlayer (from 1 to 18 monolayers) by using a one-dimensional pseudopotential for the entire overlayer-substrate system in the framework of density functional theory within the local density approximation. The elastic (energy-conserving resonant electron transfer) contribution to the total lifetime broadening of quantum well resonances has been calculated within the wave packet propagation method. The inelastic electron-electron (many-body) contribution to the lifetime broadening of both occupied and unoccupied quantum well states has been evaluated using $GW$ approximation. The decay mechanisms of both quantum well states and quantum well resonances in thick overlayers are discussed." @default.
- W2024953935 created "2016-06-24" @default.
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- W2024953935 date "2009-09-21" @default.
- W2024953935 modified "2023-10-14" @default.
- W2024953935 title "Lifetimes of quantum well states and resonances in Pb overlayers on Cu(111)" @default.
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- W2024953935 doi "https://doi.org/10.1103/physrevb.80.115425" @default.
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