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• W2025231644 abstract "The temperature/pressure phase diagram for ${(mathrm{TMTTF})}_{2}{mathrm{SbF}}_{6}$ is determined using $^{13}mathrm{C}$ NMR spectroscopy. At ambient pressure, a transition to a charge-ordered (CO) state occurs at ${T}_{mathrm{CO}}=156phantom{rule{0.3em}{0ex}}mathrm{K}$, and antiferromagnetic (AF) order is observed below ${T}_{N}=8phantom{rule{0.3em}{0ex}}mathrm{K}$. Both are suppressed with pressure: when $P>0.5phantom{rule{0.3em}{0ex}}mathrm{GPa}$, there is no evidence for CO, and the low-temperature $^{13}mathrm{C}$ NMR spectrum is consistent with a singlet [spin-Peierls (SP)] ground state. At a given pressure, the temperature dependence of the CO order parameter is not monotonic, and provides an opportunity to identify what processes could be controlling the CO amplitude. $^{19}mathrm{F}$ NMR spectroscopy provides empirical evidence that electron-counterion coupling is crucial to stabilizing the CO and AF phases." @default.
• W2025231644 created "2016-06-24" @default.
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• W2025231644 date "2004-09-08" @default.
• W2025231644 modified "2023-10-16" @default.
• W2025231644 title "Electron-lattice coupling and broken symmetries of the molecular salt<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:mrow><mml:msub><mml:mrow><mml:mo>(</mml:mo><mml:mi>TMTTF</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn>2</mml:mn></mml:msub></mml:mrow><mml:msub><mml:mi>SbF</mml:mi><mml:mn>6</mml:mn></mml:msub></mml:mrow></mml:math>" @default.
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• W2025231644 doi "https://doi.org/10.1103/physrevb.70.121101" @default.
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