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• W2025235027 abstract "Pressure-volume-temperature data, along with dielectric relaxation measurements, are reported for a series of polychlorinated biphenyls (PCB), differing in the number of chlorine atoms on their phenyl rings. Analysis of the results reveals that with increasing chlorine content, the relaxation times of the PCB become governed to a greater degree by density ρ relative to the effect of temperature T. This result is consistent with the respective magnitudes of the scaling exponent γ yielding superpositioning of the relaxation times measured at various temperatures and pressures, when plotted versus ργ∕T. While at constant (atmospheric) pressure, fragilities for the various PCB are equivalent, the fragility at constant volume varies inversely with chlorine content. Evidently, the presence of bulkier chlorine atoms on the phenyl rings magnifies the effect which the density has on the relaxation dynamics." @default.
• W2025235027 created "2016-06-24" @default.
• W2025235027 creator A5036725105 @default.
• W2025235027 creator A5073487224 @default.
• W2025235027 date "2005-04-01" @default.
• W2025235027 modified "2023-10-04" @default.
• W2025235027 title "Effect of chemical structure on the isobaric and isochoric fragility in polychlorinated biphenyls" @default.
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• W2025235027 doi "https://doi.org/10.1063/1.1863173" @default.
• W2025235027 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/15847479" @default.
• W2025235027 hasPublicationYear "2005" @default.
• W2025235027 type Work @default.
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