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• W2025261712 abstract "The strong-field response of molecules exhibits interference effects due to the geometric and electronic structure of the molecules and provides a basis for ultrafast imaging of molecular structure. This is demonstrated for high-order harmonic generation and high-order above-threshold ionization in aligned molecules by numerical solution of the time-dependent Schrödinger equation. Experimental and theoretical results for high-order harmonic generation with aligned CO2 molecules show that the harmonics exhibit an orientation dependence that is explained by the valence orbital symmetry. A detailed discussion of phase-matching effects due to the presence of different molecular orientations in an ensemble of imperfectly aligned molecules is presented." @default.
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• W2025261712 date "2005-01-20" @default.
• W2025261712 modified "2023-10-18" @default.
• W2025261712 title "Signatures of molecular structure in the strong-field response of aligned molecules" @default.
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• W2025261712 doi "https://doi.org/10.1080/09500340410001731039" @default.
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