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• W2025414424 abstract "Attachment of free, low-energy electrons to dinitrobenzene (DNB) in the gas phase leads to DNB− as well as several fragment anions. DNB−, (DNB-H)−, (DNB-NO)−, (DNB-2NO)−, and (DNB-NO2)− are found to undergo metastable (unimolecular) dissociation. A rich pattern of resonances in the yield of these metastable reactions versus electron energy is observed; some resonances are highly isomer-specific. Most metastable reactions are accompanied by large average kinetic energy releases (KER) that range from 0.5 to 1.32 eV, typical of complex rearrangement reactions, but (1,3-DNB-H)− features a resonance with a KER of only 0.06 eV for loss of NO. (1,3-DNB-NO)− offers a rare example of a sequential metastable reaction, namely, loss of NO followed by loss of CO to yield C5H4O− with a large KER of 1.32 eV. The G4(MP2) method is applied to compute adiabatic electron affinities and reaction energies for several of the observed metastable channels." @default.
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• W2025414424 date "2010-12-28" @default.
• W2025414424 modified "2023-09-26" @default.
• W2025414424 title "Metastable anions of dinitrobenzene: Resonances for electron attachment and kinetic energy release" @default.
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• W2025414424 doi "https://doi.org/10.1063/1.3514931" @default.
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