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- W2025482303 abstract "1. The ceruloplasmin-catalyzed oxidation of p-phenylenediamine and other related compounds was studied spectrophotometrically and manometrically. 2. For p-phenylenediamine, the reaction sequence proceeded through three stages. The first probably involved the formation of a charge-transfer complex between substrate and ceruloplasmin Cu2+. The second involved the transfer of a single electron from substrate to Cu2+ to form a yellow free radical, as determined using electron paramagnetic resonance techniques. The third step involved the loss of another electron from the yellow free radical, either through a disproportionation process or by reaction with enzyme, to form a short-lived diradical species that reacted with more p-phenylenediamine to form a stable purple product. 3. The purple product formed in p-phenylenediamine oxidation can act as an inhibitor for the oxidation of p-phenylenediamine and other substrates. 4. The oxidative sequence of durenediamine was similar to that for p-phenylenediamine, except here the diradical that formed rearranged and hydrolyzed in water to form duroquinone and ammonia." @default.
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- W2025482303 date "1963-01-01" @default.
- W2025482303 modified "2023-09-26" @default.
- W2025482303 title "On the mechanism of ceruloplasmin-catalyzed oxidations" @default.
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- W2025482303 doi "https://doi.org/10.1016/0006-3002(63)90546-8" @default.
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