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• W2025497771 endingPage "015302" @default.
• W2025497771 startingPage "015302" @default.
• W2025497771 abstract "Exactly solvable reference potentials of several smoothly joined Morse-type components were constructed for the lowest two excimer states of the Ar2 molecule. The parameters of the potentials have been ascertained by fitting to the experimental data, and they are reliable in a wide range of nuclear separations (r≥1.9 A). A large number of quantum mechanical Franck–Condon factors for the 0u+→ 0g+ and 1u→ 0g+ transitions have been calculated and compared with the observed spectroscopic features. The fitting procedure also involved dipole transition moments, which have been adjusted to the known radiative lifetimes of the vibrational levels. The resulting potential energy curves accurately reproduce the first and the second emission continua of Ar2* as well as the oscillatory spectrum related to their inner turning point region. The numbering and the positions of the vibrational levels reported by Herman et al (1988 J. Chem. Phys. 89 4535) have been confirmed. The calculated spectroscopic parameters, ωe=296.26 cm−1, De=6128.3 cm−1 for the 0u+ state and ωe=287.30 cm−1, De=5929.6 cm−1 for the 1u state, are consistent with previous estimations. Separation between the minima of the potential wells at Re=2.3893 A was found to be 416.1 cm−1 (51.59 meV), compared with 606.8 cm−1 (75.24 meV) splitting in the separated-atom limit." @default.
• W2025497771 created "2016-06-24" @default.
• W2025497771 creator A5016165151 @default.
• W2025497771 date "2007-12-12" @default.
• W2025497771 modified "2023-09-27" @default.
• W2025497771 title "Potential energy curves and transition probabilities for the excimer states 0_u⁺(³P₁) and 1_u(³P₂) of Ar₂" @default.
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• W2025497771 doi "https://doi.org/10.1088/0031-8949/77/01/015302" @default.
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