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- W2025506329 abstract "The photophysical properties of the Ru(bpy)2+3 complex incorporated into swelled Nafion membrane have been re-investigated with attention to the problem of partitioning of the luminescence complex between different microdomains of the membrane. The luminescence decay profiles obtained at different emission wavelengths and temperatures are studied by single curve, and global analysis methods. At low concentration of the probe in the membrane, the luminescence decay surface follows a biexponential law with normalized amplitudes strongly dependent on the emission wavelength. The shorter lifetime component appears more significantly in the high-energy part of the luminescence spectrum. The recovering of two average lifetimes obtained from global biexponential fitting indicates that two major microdomains for the probe are in the membrane. The first one related to the short lifetime is ascribed to the fraction of probe embeded by the perfluorinated ether environment while the second microdomain is the heterogeneous water cluster interface which gives the long-lived lifetime component of the complex in Nafion." @default.
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- W2025506329 date "1998-07-01" @default.
- W2025506329 modified "2023-10-16" @default.
- W2025506329 title "Inhomogeneous decay kinetics of Ru(bpy)2+3 incorporated into nafion film" @default.
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- W2025506329 doi "https://doi.org/10.1016/s0022-2313(98)00016-7" @default.
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