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- W2025517581 abstract "An analysis of electrical effects associated with the operation of thickness-shear-mode acoustic wave sensors in liquid is presented. A frequent observation found for this system is that the magnitude and the sign of frequency changes cannot be explained by the previously developed mass- and the viscous-loading formulations. These discrepancies are attributed, in part, to the electric properties of the liquid layers in the vicinity of the device electrode. Using network analysis, the resonance frequencies and the equivalent circuit parameters of the device were monitored for a variety of electrolytes in the concentration range 1 to 3000 mM. A nonlinear and periodic dependence was found between both the series resonance frequency and the motional resistance parameter of the device with respect to concentration of electrolyte. Unlike the case of viscous-loading of the sensor, which is known to exhibit a linear and inversely proportional relationship between frequency change and motional resistance, the electrolyte loading of the device yields an unexpected spiral dependence of the two quantities. The spiral dependence provides further proof for the periodicity of the dependence of the series resonance frequency and motional resistance parameter on electrolyte concentration. This finding has important implications for the development of acoustic wave biosensors, since solutions of biochemical species usually involve electrolytes of variable composition, which may affect the electrical double layer structure and, in turn, the response of the sensor." @default.
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- W2025517581 date "2000-03-01" @default.
- W2025517581 modified "2023-09-26" @default.
- W2025517581 title "Interfacial Properties and the Response of the Transverse Acoustic Wave Device in Electrolytes" @default.
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- W2025517581 doi "https://doi.org/10.1002/(sici)1521-4109(20000301)12:5<326::aid-elan326>3.0.co;2-a" @default.
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