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- W2025549706 abstract "The DOOO radical has been produced by three-body association between OD and O2 in a supersonic free-jet expansion and investigated using action spectroscopy, an IR-UV double-resonance technique. Partially rotationally structured bands observed at 2635.06 and 5182.42 cm(-1) are assigned to the OD stretch fundamental (nu(OD)) and overtone (2nu(OD)), respectively, of the trans-DOOO radical. Unstructured bands observed in both spectral regions are assigned to cis-DOOO. Nascent OD X(2)Pi product state distributions following vibrational predissociation appear to be nearly statistical with respect to the degree of rotational excitation, but display a marked propensity for Pi(A') Lambda-doublets, which is interpreted as a signature of a planar dissociation. The energetically highest open OD X(2)Pi product channel implies an upper limit dissociation energy D0 < or = 1856 cm(-1) or 5.31 kcal mol(-1). This value allows refinement of the upper limit D0 of the atmospherically important HOOO isotopomer, suggesting that it is marginally less stable than previously thought." @default.
- W2025549706 created "2016-06-24" @default.
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- W2025549706 date "2008-05-29" @default.
- W2025549706 modified "2023-09-23" @default.
- W2025549706 title "Infrared Action Spectroscopy of the OD Stretch Fundamental and Overtone Transitions of the DOOO Radical" @default.
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- W2025549706 doi "https://doi.org/10.1021/jp801232a" @default.
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