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• W2025647002 startingPage "64" @default.
• W2025647002 abstract "Triazine herbicides detected in surface and groundwater pose environmental and health risks. Removal of triazine herbicides (simazine, atrazine and terbuthylazine) by polymer-clay composites was studied and modeled. Their binding by a poly 4-vinyl pyridine co styrene-montmorillonite (HPVP-CoS-MMT) composite was especially high due to specific interactions between the herbicides and polymer, mainly hydrogen bonds and π-π stacking. The binding kinetics to the composite was in the order of simazine > atrazine > terbuthylazine, which was in accord with their equilibrium Langmuir binding coefficients; 44,000, 17,500 and 16,500 M(-1), respectively, which correlated with herbicide accessibility to form specific interaction with the polymer. Simazine binding kinetics to the composite was significantly faster than to granulated activated carbon (GAC), reaching 93% vs 38% of the maximal adsorption within 10 min, respectively. Herbicide filtration by composite columns was adequately fitted by a model which considers convection and employs Langmuir formalism for kinetics of adsorption/desorption. Filtration of simazine (10 μg L(-1)) by composite columns (40 cm long, which included 26 g composite mixed with sand 1:40 (weight ratio)), was well predicted by the model with nearly 120 L purified, i.e., effluent concentrations were below regulation limit (3 μg L(-1)). Effluent concentrations from GAC columns exceeded the limit after filtering 5 L. Experimental results and model predictions suggest that while GAC has a high capacity for simazine binding, the composite has higher affinity towards the herbicide and its adsorption is faster, which yields more efficient filtration by composite columns." @default.
• W2025647002 created "2016-06-24" @default.
• W2025647002 creator A5029151977 @default.
• W2025647002 creator A5040840781 @default.
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• W2025647002 date "2015-03-01" @default.
• W2025647002 modified "2023-09-25" @default.
• W2025647002 title "Filtration of triazine herbicides by polymer-clay sorbents: Coupling an experimental mechanistic approach with empirical modeling" @default.
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• W2025647002 doi "https://doi.org/10.1016/j.watres.2014.11.032" @default.
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