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- W2025849176 abstract "Photodissociation spectroscopy is applied to benzene cluster ions in ultraviolet and infrared regions. In the ultraviolet photodissociation spectrum of (C6H6)3+ , a characteristic broad band emerges at 255 nm. This band is assigned to a π*←π transition of a solvent benzene molecule that exists in the trimer. This is in accordance with the previous model of the ion cluster with a dimer ion core and a solvent benzene molecule. The infrared photodissociation spectra of (C6H6)n+ (n=3–5) show a sharp band at 3066 cm−1. The band is attributed to a C–H stretching vibration of the dimer ion core. The infrared spectra of (C6H6)n+ (n=3–5) are fitted to the model spectra reproduced by combining the C–H stretching bands of the dimer ion core and the solvent benzene molecule. The infrared photodissociation spectra of mixed benzene trimer ions with one or two benzene-d6 molecules demonstrate that there is no correlation between the excited dimer ion core site in the trimer and the photofragment dimer ion species. This implies that a dimer ion core switching occurs in photoexcited vibrational states prior to the dissociation." @default.
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- W2025849176 date "2001-04-22" @default.
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- W2025849176 title "Photodissociation spectroscopy of benzene cluster ions in ultraviolet and infrared regions: Static and dynamic behavior of positive charge in cluster ions" @default.
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- W2025849176 doi "https://doi.org/10.1063/1.1359446" @default.
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