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• W2026178009 abstract "Abstract This article completes our comprehensive understanding of the electron transport properties of our original π‐conjugated redox‐active molecular wires comprising Fe bridged by p ‐phenylene linkers (tpy=2,2′:6′,2′′‐terpyridine). The Fe(tpy) 2 oligomer wires comprise three types of tpy ligands: the anchor tpy ligand ( A series) makes a junction between the wire and electrode, the bridging bis‐tpy ligand ( L series) connects the Fe(tpy) 2 units, and the terminal tpy ligand ( T series) possesses a redox site as a probe for the long‐range electron transport ability. Taking advantage of the precise tunability of the composition of the Fe(tpy) 2 oligomer wires, thus far we investigated how A and L impacted on the electron‐transport ability. The excellent long‐range electron transport ability with ultrasmall attenuation constants ( β d , 0.002 Å −1 as the minimum) depends on L significantly [ Chem. Asian J. 2009 , 4 , 1361], whereas A is unrelated to the β d value, but influences the zero‐distance electron‐transfer rate constant, k et 0 [ J. Am. Chem. Soc. 2010 , 132 , 4524]. Herein we study the influence of terminal ligand T x ( x =1–3). β d is independent of T , however, T 3 , with a cyclometallated Ru complex as the redox site, gives rise to a k et 0 value greater than T 1 and T 2 with ferrocene. This series of simple but definitive conclusions indicates that we have reached the stage of being able to precisely design molecular wires to attain desirable single‐molecule electron conduction." @default.
• W2026178009 created "2016-06-24" @default.
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• W2026178009 date "2013-02-19" @default.
• W2026178009 modified "2023-10-18" @default.
• W2026178009 title "Terminal Redox-Site Effect on the Long-Range Electron Conduction of Fe(tpy)₂Oligomer Wires on a Gold Electrode" @default.
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• W2026178009 doi "https://doi.org/10.1002/chem.201203913" @default.
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