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• W2026258501 abstract "Structural changes of silver terrace domains in aqueous perchloric acid solution at constant anodic current density (j) and room temperature were followed by in situ scanning tunneling microscopy sequential imaging. For j15 ensuremath{mu}A ${mathrm{cm}}^{mathrm{ensuremath{-}}2}$ silver electrodissolution proceeds at step edges without roughening. Conversely, for jensuremath{gtrsim}15 ensuremath{mu}A ${mathrm{cm}}^{mathrm{ensuremath{-}}2}$ the silver surface becomes progressively rougher to attain, after a certain critical time, a steady roughness. In this case, the dynamic scaling theory applied to STM images indicates that the dissolving silver surface can be described as a self-affine fractal surface with a static roughening exponent ensuremath{alpha}=0.90ifmmodepmelsetextpmfi{}0.06, and a dynamic roughening exponent ensuremath{beta}=0.36ifmmodepmelsetextpmfi{}0.08. The value of ensuremath{alpha} is consistent with the relevant role played by surface diffusion in the silver electrodissolution mechanism, whereas the value of ensuremath{beta} is slightly higher than those derived from growth models incorporating surface diffusion. The difference in the value of ensuremath{beta} would reflect the influence of either the electric field or energetic barriers at step edges on the rate of roughness development. textcopyright{} 1996 The American Physical Society." @default.
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• W2026258501 date "1996-04-15" @default.
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• W2026258501 title "<i>In</i><i>situ</i>sequential STM imaging of structural changes resulting from the electrodissolution of silver crystal surfaces in aqueous perchloric acid: The roughening kinetics" @default.
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• W2026258501 doi "https://doi.org/10.1103/physrevb.53.10217" @default.
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