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- W2026371692 abstract "We study the behaviour of a molecular excited electron experiencing the quantum superposition of the ground- and excited-state molecular orientation, as well as the rotating nuclear frame. The theoretical description of this `average free orientational polarizability' is presented for a short optical Fourier-limited pulse whose large spectral bandwidth overlaps N rotational states in the excited electronic-vibrational state. This pulse induces within the rotational structure a diffraction grating and provides the excited electron wavefunction with a characteristic interference pattern. We derive the explicit expression of the `diffracted-electron induced dipole' and investigate the rotational motion of the excited molecule." @default.
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- W2026371692 date "2002-03-26" @default.
- W2026371692 modified "2023-10-18" @default.
- W2026371692 title "Orientational polarizability and diffracted-molecular-electron induced dipole" @default.
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- W2026371692 doi "https://doi.org/10.1088/0953-4075/35/7/306" @default.
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